Quantum and semiclassical dynamics of differential optical collisions

Rebentrost, F. ; Klose, S. ; Grosser, J.
Springer
Published 1998
ISSN:
1434-6079
Keywords:
PACS. 32.70.-n Intensities and shapes of atomic spectral lines - 34.20.Cf Interatomic potentials and forces - 34.50.Rk Laser modified scattering and reactions
Source:
Springer Online Journal Archives 1860-2000
Topics:
Physics
Notes:
Abstract: We apply quantum and semiclassical theories to differential optical collisions Na(32S1/2) + Kr + Na(32P1/2,3/2) + Kr. Our results provide a basis to analyze recent experiments in which for the first time optical collisions were investigated with angular resolution under crossed-beam conditions. A characteristic feature of the differential cross sections is the pronounced oscillatory structure due to interferences of different Condon paths. These Stueckelberg oscillations form an extremely sensitive probe of the collisional dynamics and of the molecular interactions. We demonstrate perspectives to determine geometric properties of the collision complex by excitation with polarized light. By final state analysis nonadiabatic (spin-orbit, rotational) interactions can be studied with complete control of the path. In summary it is shown that the method of differential detection of optical collisions opens a variety of new accesses to atomic and molecular subcollisions.
Type of Medium:
Electronic Resource
URL:
_version_ 1798297641398829056
autor Rebentrost, F.
Klose, S.
Grosser, J.
autorsonst Rebentrost, F.
Klose, S.
Grosser, J.
book_url http://dx.doi.org/10.1007/s100530050094
datenlieferant nat_lic_papers
hauptsatz hsatz_simple
identnr NLM189694319
issn 1434-6079
journal_name The European physical journal
materialart 1
notes Abstract: We apply quantum and semiclassical theories to differential optical collisions Na(32S1/2) + Kr + Na(32P1/2,3/2) + Kr. Our results provide a basis to analyze recent experiments in which for the first time optical collisions were investigated with angular resolution under crossed-beam conditions. A characteristic feature of the differential cross sections is the pronounced oscillatory structure due to interferences of different Condon paths. These Stueckelberg oscillations form an extremely sensitive probe of the collisional dynamics and of the molecular interactions. We demonstrate perspectives to determine geometric properties of the collision complex by excitation with polarized light. By final state analysis nonadiabatic (spin-orbit, rotational) interactions can be studied with complete control of the path. In summary it is shown that the method of differential detection of optical collisions opens a variety of new accesses to atomic and molecular subcollisions.
package_name Springer
publikationsjahr_anzeige 1998
publikationsjahr_facette 1998
publikationsjahr_intervall 8004:1995-1999
publikationsjahr_sort 1998
publisher Springer
reference 1 (1998), S. 277-289
schlagwort PACS. 32.70.-n Intensities and shapes of atomic spectral lines - 34.20.Cf Interatomic potentials and forces - 34.50.Rk Laser modified scattering and reactions
search_space articles
shingle_author_1 Rebentrost, F.
Klose, S.
Grosser, J.
shingle_author_2 Rebentrost, F.
Klose, S.
Grosser, J.
shingle_author_3 Rebentrost, F.
Klose, S.
Grosser, J.
shingle_author_4 Rebentrost, F.
Klose, S.
Grosser, J.
shingle_catch_all_1 Rebentrost, F.
Klose, S.
Grosser, J.
Quantum and semiclassical dynamics of differential optical collisions
PACS. 32.70.-n Intensities and shapes of atomic spectral lines - 34.20.Cf Interatomic potentials and forces - 34.50.Rk Laser modified scattering and reactions
PACS. 32.70.-n Intensities and shapes of atomic spectral lines - 34.20.Cf Interatomic potentials and forces - 34.50.Rk Laser modified scattering and reactions
Abstract: We apply quantum and semiclassical theories to differential optical collisions Na(32S1/2) + Kr + Na(32P1/2,3/2) + Kr. Our results provide a basis to analyze recent experiments in which for the first time optical collisions were investigated with angular resolution under crossed-beam conditions. A characteristic feature of the differential cross sections is the pronounced oscillatory structure due to interferences of different Condon paths. These Stueckelberg oscillations form an extremely sensitive probe of the collisional dynamics and of the molecular interactions. We demonstrate perspectives to determine geometric properties of the collision complex by excitation with polarized light. By final state analysis nonadiabatic (spin-orbit, rotational) interactions can be studied with complete control of the path. In summary it is shown that the method of differential detection of optical collisions opens a variety of new accesses to atomic and molecular subcollisions.
1434-6079
14346079
Springer
shingle_catch_all_2 Rebentrost, F.
Klose, S.
Grosser, J.
Quantum and semiclassical dynamics of differential optical collisions
PACS. 32.70.-n Intensities and shapes of atomic spectral lines - 34.20.Cf Interatomic potentials and forces - 34.50.Rk Laser modified scattering and reactions
PACS. 32.70.-n Intensities and shapes of atomic spectral lines - 34.20.Cf Interatomic potentials and forces - 34.50.Rk Laser modified scattering and reactions
Abstract: We apply quantum and semiclassical theories to differential optical collisions Na(32S1/2) + Kr + Na(32P1/2,3/2) + Kr. Our results provide a basis to analyze recent experiments in which for the first time optical collisions were investigated with angular resolution under crossed-beam conditions. A characteristic feature of the differential cross sections is the pronounced oscillatory structure due to interferences of different Condon paths. These Stueckelberg oscillations form an extremely sensitive probe of the collisional dynamics and of the molecular interactions. We demonstrate perspectives to determine geometric properties of the collision complex by excitation with polarized light. By final state analysis nonadiabatic (spin-orbit, rotational) interactions can be studied with complete control of the path. In summary it is shown that the method of differential detection of optical collisions opens a variety of new accesses to atomic and molecular subcollisions.
1434-6079
14346079
Springer
shingle_catch_all_3 Rebentrost, F.
Klose, S.
Grosser, J.
Quantum and semiclassical dynamics of differential optical collisions
PACS. 32.70.-n Intensities and shapes of atomic spectral lines - 34.20.Cf Interatomic potentials and forces - 34.50.Rk Laser modified scattering and reactions
PACS. 32.70.-n Intensities and shapes of atomic spectral lines - 34.20.Cf Interatomic potentials and forces - 34.50.Rk Laser modified scattering and reactions
Abstract: We apply quantum and semiclassical theories to differential optical collisions Na(32S1/2) + Kr + Na(32P1/2,3/2) + Kr. Our results provide a basis to analyze recent experiments in which for the first time optical collisions were investigated with angular resolution under crossed-beam conditions. A characteristic feature of the differential cross sections is the pronounced oscillatory structure due to interferences of different Condon paths. These Stueckelberg oscillations form an extremely sensitive probe of the collisional dynamics and of the molecular interactions. We demonstrate perspectives to determine geometric properties of the collision complex by excitation with polarized light. By final state analysis nonadiabatic (spin-orbit, rotational) interactions can be studied with complete control of the path. In summary it is shown that the method of differential detection of optical collisions opens a variety of new accesses to atomic and molecular subcollisions.
1434-6079
14346079
Springer
shingle_catch_all_4 Rebentrost, F.
Klose, S.
Grosser, J.
Quantum and semiclassical dynamics of differential optical collisions
PACS. 32.70.-n Intensities and shapes of atomic spectral lines - 34.20.Cf Interatomic potentials and forces - 34.50.Rk Laser modified scattering and reactions
PACS. 32.70.-n Intensities and shapes of atomic spectral lines - 34.20.Cf Interatomic potentials and forces - 34.50.Rk Laser modified scattering and reactions
Abstract: We apply quantum and semiclassical theories to differential optical collisions Na(32S1/2) + Kr + Na(32P1/2,3/2) + Kr. Our results provide a basis to analyze recent experiments in which for the first time optical collisions were investigated with angular resolution under crossed-beam conditions. A characteristic feature of the differential cross sections is the pronounced oscillatory structure due to interferences of different Condon paths. These Stueckelberg oscillations form an extremely sensitive probe of the collisional dynamics and of the molecular interactions. We demonstrate perspectives to determine geometric properties of the collision complex by excitation with polarized light. By final state analysis nonadiabatic (spin-orbit, rotational) interactions can be studied with complete control of the path. In summary it is shown that the method of differential detection of optical collisions opens a variety of new accesses to atomic and molecular subcollisions.
1434-6079
14346079
Springer
shingle_title_1 Quantum and semiclassical dynamics of differential optical collisions
shingle_title_2 Quantum and semiclassical dynamics of differential optical collisions
shingle_title_3 Quantum and semiclassical dynamics of differential optical collisions
shingle_title_4 Quantum and semiclassical dynamics of differential optical collisions
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timestamp 2024-05-06T10:11:13.740Z
titel Quantum and semiclassical dynamics of differential optical collisions
titel_suche Quantum and semiclassical dynamics of differential optical collisions
topic U
uid nat_lic_papers_NLM189694319